•  
  •  
 
CHEMISTRY AND CHEMICAL ENGINEERING

Abstract

The purpose of the research is to develop a method of synthesizing new acetylene diols, to determine their structure, physico-chemical properties and to create optimal conditions by studying the effect of various environments on product yield. For the first time, nucleophilic coupling reactions of 1-ethynylcyclohexanol with some ketones - cyclohexanone, acetophenone, para-chloroacetophenone, adamantanone, methylhexylketone and ethyl-n-butyl ketones were studied using the Bu4NOH/DMSO/H2O catalytic system. New acetylene diols – 1-(2-(1-hydro-xycyclohexyl)ethynyl)cyclohexanol (1), 1-(3-hydroxy-3-phenylbut-1-ynyl)cyclohexanol (2), 1-(3-(4-chlorophenyl)-3-hydroxybut-1-ynyl)cyclo-hexanol(3), 1-(2-(1-hydroxyadamantanyl)-ethynyl)cyclohexanol (4), 1-(3-hydroxy-3-methyldec-1-ynyl)cyclohexanol(5) and 1-(3-ethyl-3-hydroxyhept-1-ynyl)cyclohexanol (6) were synthesized in the process. The effects of the catalyst for the synthesis of acetylene diols, the nature of the solvent, the mole ratio of the starting materials, the temperature, and the duration of the reaction were systematically analyzed. The composition, structure and purity of the synthesized acetylene diols were determined by modern physical and chemical research methods.

Share

COinS
 
 

To view the content in your browser, please download Adobe Reader or, alternately,
you may Download the file to your hard drive.

NOTE: The latest versions of Adobe Reader do not support viewing PDF files within Firefox on Mac OS and if you are using a modern (Intel) Mac, there is no official plugin for viewing PDF files within the browser window.