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CHEMISTRY AND CHEMICAL ENGINEERING

Abstract

In this study, the kinetic characteristics of the nucleophilic substitution (SN2) reaction between piperidine and chloroacetic acid were investigated in real time at 50, 60, and 70 °C using ATR-FTIR spectroscopy. The spectral analysis revealed a gradual decrease in the C–Cl stretching vibration in the 710–730 cm⁻¹ region and a simultaneous increase in absorption bands corresponding to the C–N bond in the 1020–1250 cm⁻¹ region, confirming the consistent progression of the reaction. Analysis of the conversion function X(t) showed values of X = 0.669 at 50 °C, X = 0.826 at 60 °C, and X = 0.970 at 70 °C, indicating a substantial acceleration of the reaction rate with increasing temperature. The dX/dt–t profiles displayed a maximum initial reaction rate followed by exponential decay. Linear regression analysis demonstrated excellent agreement with the first-order kinetic model at all temperatures (R² = 0.97–0.999), and the rate constants increased from 0.0078 → 0.0106 → 0.0143 min⁻¹. Arrhenius analysis yielded an activation energy of 27.9 kJ·mol⁻¹. These results confirm that the piperidine–chloroacetate system proceeds via an SN2 mechanism and demonstrate that ATR-FTIR spectroscopy provides high sensitivity and accuracy for real-time monitoring of reaction processes.

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